Anion-Activated Supramolecular Proton Relays Enable Neutral-pH and Seawater Oxidation
Neutral-pH and direct seawater oxidation are critically hindered by sluggish proton-coupled electron transfer (PCET) and competitive chloride corrosion. Here, we employ surface-confined azacrown macrocycles of varying nitrogen content as supramolecular proton-management layers rather than conventional redox catalysts...