Interfacial Charge Modulation of Covalent Metal-Organic Frameworks for Efficient H2O2 Electrosynthesis.
Electrochemical H2O2 synthesis through the two-electron oxygen reduction reaction offers a sustainable alternative to the energy-intensive anthraquinone process. Crystalline porous frameworks are attractive for this route because of their structural precision, yet poor electrolyte wetting and limited electrochemical ac...