Line-narrowing spectroscopy of water-soluble chlorophyll-binding protein (WSCP) embedded in an asymmetric phonon bath.
A tractable and computationally expedient electronic transition dipole moment time-correlation function of a tetrameric photosynthetic complex binding two pigment dimers, from which nonlinear optical time- and frequency-domain signals may be obtained, and the bath spectral density, which impacts the dynamics and the sh...