Oxonium-Embedded Benzo[b]perylene: A Redox-Switchable Closed-Shell π‑Cation, and Its Paramagnetic Charge-Transfer Salt with TCNE•–
Organic cations and radicals are promising building components for organic optoelectronics, spintronics and quantum information processing. Realizing their full potential requires strategies to enhance their stability and precisely control their solid-state organization. Herein, we describe a modular synthetic strategy...