Lin Wen

Unlocking Zenith Electronic State of Ni Sites in Ligand‐Engineered COFs for Efficient •O2 −‐Driven Uranium Photoreduction

ABSTRACT Photocatalytic uranium reduction via the superoxide radical (•O2 −) pathway is a sustainable route, but its efficiency is constrained by rapid charge recombination and poor O2 activation. Herein, we develop a ligand engineering strategy to construct a series of Ni‐diketimine‐linked COFs by varying the diketone...