Engineering Metal Pyrazolate Coordination Polymers for Highly Selective Direct Air Capture via Metal–Ligand Cooperativity and Moisture-Gated Mechanism
Direct air capture (DAC) of CO2 has emerged as an indispensable negative emission technology, yet current sorbents remain constrained by the persistent trade-off between intrinsic capture capacity and regeneration energy alongside the extrinsic challenge of atmospheric moisture inhibition. Herein, engineering of crysta...