Hydrogen spillover can decouple elementary steps in the hydrogen evolution reaction (HER), yet conventional bimetallic catalysts often suffer from discontinuous interfaces that block spillover pathways. Herein, an interfacial hydrogen spillover mechanism is engineered in a Pd-PdNi-Ni catalyst via a partial interface al...
Di Wang, Jun Mei, Qian-Qian Yao et al.· Angewandte Chemie· 0 citations
Layered oxide cathodes have attracted worldwide attention due to environmentally friendliness, structural diversity, and economic benefits. However, poor long-term cycling and unsatisfactory rate performance hinder the practical application. Hence, an oxide cathode with self-adaptive volume has been designed, achieving...
Jia-Yang Li, Ying Guo, Xin Wang et al.· Nature Communications· 0 citations
Solid‐state lithium metal batteries are promising next generation energy storage devices and composite solid electrolytes (CSEs) with high ionic conductivity and mechanical stability have attracted widespread attention. However, the slow ion transport kinetics at the heterogeneous interface between ceramic fillers and...
Kan Zhao, Lin Li, Bo Wang et al.· Advanced Functional Material...· 0 citations
Sodium-metal batteries (SMBs) exhibit high theoretical specific capacity and take advantage of sodium's natural abundance and low cost, showing great promise for broad next-generation energy-storage applications. In this review, we summarize the major practical bottlenecks restricting SMB development. The solid-electro...
Sikandar Iqbal, U. Ghani, Xue-Bing Zhu et al.· Advances in Materials· 0 citations
Strain engineering offers a powerful means to regulate the electronic structure and catalytic behavior of active metal sites, yet a general framework linking strain to electrocatalytic performance remains elusive beyond the conventional d-band model. Here we report crumpled double-transition-metal MXene nanosheets (Mo2...
Xiao-Min Chen, Ding Yuan, Chao Rong et al.· Advances in Materials· 1 citation
High-energy-density lithium-metal batteries (LMBs) are promising for next-generation energy storage, but their practical application is hindered by lithium dendrite growth and electrolyte interfacial instability under high-voltage conditions. Here, we report a molecule-reconstruction strategy to regulate Li+ solvation...
Yan-Xin Jiang, Yan Su, Guo-Qiang He et al.· Angewandte Chemie· 0 citations
Electrocatalytic nitrogen reduction reaction (eNRR) under ambient conditions is a promising route for sustainable ammonia synthesis, yet its progress is fundamentally limited by the inertness of N≡N bonds and the lack of robust, selective catalysts. Here, we report the first synthesis of a rutile‐structured high‐en...
Yiwen Su, Xin-Zhong Wang, Jin-jin Wu et al.· Advanced Functional Material...· 0 citations
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