Decoupling the activity-selectivity trade-off via synergistic dual-site electrocatalysis to steer CN coupling selectivity toward urea electrosynthesis.
Electrosynthesis of urea holds promise for carbon mitigation, pollutant valorization, and green chemical production, yet it is hindered by competitive adsorption and sluggish CN coupling. Here, we develop a dual-single-atom catalyst, wherein Fe and Ni are atomically dispersed on a CeO2 support (Fe3Ni1-CeO2). By spatial...