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Sep 2026

Decoupling the activity-selectivity trade-off via synergistic dual-site electrocatalysis to steer CN coupling selectivity toward urea electrosynthesis.

Electrosynthesis of urea holds promise for carbon mitigation, pollutant valorization, and green chemical production, yet it is hindered by competitive adsorption and sluggish CN coupling. Here, we develop a dual-single-atom catalyst, wherein Fe and Ni are atomically dispersed on a CeO2 support (Fe3Ni1-CeO2). By spatial...

Fan Wu, Rui-Jie Zhou, Jun-Rong Zou et al. · 0 citations
Aug 2026

Isotopological Modulation of Entanglement in 3D Covalent Organic Frameworks Unlocks a Fully Open Catalytic Architecture.

Rational control over structural entanglement in three-dimensional covalent organic frameworks (3D COFs) is essential for optimizing catalytic-site accessibility and substrate transport in heterogeneous catalysis. However, conventional thermodynamically governed crystallization often produces interpenetrated architectu...

Hao Wang, Cheng-Tao Gong, Yuan-Hui Yao et al. · 0 citations

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