Electrode–electrolyte interfacial microenvironments (EEIMs) critically govern the performance of electrochemical CO2 reduction (ECR). However, the potential-driven dynamic distribution of interfacial cations and their reshaping effects on the interfacial water structure and proton-coupled electron transfer kinetics r...
Hang Wang, Chuan-Jun Wang, Long Ma et al.· ACS Catalysis· 1 citation
Achieving efficient C–C coupling in photocatalytic CO2 reduction is fundamentally limited by the inability of semiconductor surfaces to simultaneously stabilize and differentiate key intermediates (*CO and *CHO). In this work, we establish an asymmetric Cu valence engineering strategy in tetragonal CuInS2 that enable...
Hang Zhao, Ren-Jie Bi, Ming-Dong Ju et al.· ACS Catalysis· 0 citations
Acidic electrocatalytic CO2 reduction (CO2RR) can mitigate carbonate crossover and deposition issues inherent in conventional neutral/alkaline systems, yet it faces the dual challenges of severe hydrogen evolution reaction (HER) competition and local salt precipitation that deactivates electrodes. To address these is...
Chuan-Jun Wang, Cai Chen, Gui Zhou et al.· Journal of Physical Chemistr...· 0 citations
This study proposed a new strategy for simultaneous catalytic conversion of wheat straw with a deep eutectic solvent-assisted ball milling method at high solid content (20%) conditions, thereby improving monosaccharide yield and exergy efficiency. After mechanical shearing by ball milling, the crystallinity of wheat...
Xian-Wu Tan, Ao Xia, Xian-Qing Zhu et al.· Industrial & Engineering...· 0 citations
Electrochemical CO2 reduction (ECR) is highly sensitive to the electrode-electrolyte interfacial microenvironment (EEIM). However, how the hydration structures of alkali-metal cations reorganize EEIM and thereby influence the energetics of ECR and hydrogen evolution reaction (HER) related elementary steps remains unc...
Hang Wang, Yuan-Chang Liang, Chuan-Jun Wang et al.· Journal of Physical Chemistr...· 0 citations
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