Covalent-Organic Framework-Manipulated Multi-Reactant Activation Enables Polystyrene Electrodegradation in Tandem With Over-Oxidation Product Upgrading.
Polystyrene (PS) waste is exceptionally difficult to chemically degrade under environmental conditions, and the high-value utilization of low-value C1 products generated during the process has never been achieved. Herein, we constructed a metalloporphyrin-anthracene sp2 covalent-organic framework (COF) electrocatalyst,...