Simulation of two-dimensional electronic and double-quantum coherence spectra of molecular polaritons.
We simulate two-dimensional electronic spectroscopy (2DES) and double-quantum coherence (DQC) signals for a dissipative Tavis-Cummings model using the third-order optical response function formalism. Cavity photon loss, excited state population relaxation, and fast dephasing are included through Lindblad terms, while s...