Zhen Wang

Spin State Crossover of an Fe1 Single-Atom Catalyst for Promoted Methane Conversion to Oxygenates under Mild Conditions

Engineering the electronic and spin states of active centers for promoted oxygenate production from methane remains a fundamental challenge in catalysis. Herein, we demonstrate that spin crossover of Fe1 single-atoms from high spin (HS) to low spin (LS) could boost the oxygenate yield by 5.3-fold. The spin transition...